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Enhanced quantum yield of nitrogen fixation for hydrogen storage with in situ-formed carbonaceous radicals.
Chemical Communications : Chem Comm 2015 March 22
NH3 is a potential hydrogen energy carrier. Here we use alcohols as hole scavengers to investigate the nitrogen photofixation mechanisms including direct and indirect electron transfer processes. The t-butanol system exhibited the highest quantum yield of 36.1%, ascribing to the in situ-formed indirect electronic transmitter ˙CO2(-).
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