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Structural relaxations of thin polymer films.
Physical Review Letters 2012 June 30
Time-dependent changes of thermodynamic properties due to structural relaxations and physical aging occur in all glasses. We show that the physical aging of thin supported films of star-shaped macromolecules, with f arms of length N(arm), exhibits average aging dynamics that are sensitive to f and N(arm). Regions of the films in proximity to interfaces age at substantially different rates than the interior of the film; this is also true of linear chain systems. This behavior may be reconciled in terms of a universal picture that accounts only for changes in the local T(g) of the films.
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