Stephen K Wilke, Chris J Benmore, Oliver L G Alderman, Ganesh Sivaraman, Matthew D Ruehl, Krista L Hawthorne, Anthony Tamalonis, David A Andersson, Mark A Williamson, Richard Weber
Advances in nuclear power reactors include the use of mixed oxide fuel, containing uranium and plutonium oxides. The high-temperature behaviour and structure of PuO2-x above 1,800 K remain largely unexplored, and these conditions must be considered for reactor design and planning for the mitigation of severe accidents. Here, we measure the atomic structure of PuO2-x through the melting transition up to 3,000 ± 50 K using X-ray scattering of aerodynamically levitated and laser-beam-heated samples, with O/Pu ranging from 1...
April 26, 2024: Nature Materials