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https://www.readbyqxmd.com/read/28433818/spatial-temporal-variability-and-transportation-mechanism-of-polychlorinated-biphenyls-in-the-yangtze-river-estuary
#1
Lei Chen, Ye Yang, Jing Chen, Shuohan Gao, Shasha Qi, Cheng Sun, Zhenyao Shen
Although the variability of polychlorinated biphenyls (PCBs) is strongly dependent on the hydro-sediment pattern, the quantification of this interaction is still not well described, especially for estuary areas. In this study, both chemical analyses and numerical simulation were conducted to explain the temporal-spatial variability and transportation mechanism of PCBs in the Yangtze River Estuary (YRE). The impacts of the upstream Three Gorges Dam (TGD) on estuarine PCBs were also addressed with a simulated scenario...
April 20, 2017: Science of the Total Environment
https://www.readbyqxmd.com/read/28433504/intensification-of-ultrasonic-assisted-crude-oil-demulsification-based-on-acoustic-field-distribution-data
#2
Matheus F Pedrotti, Michele S P Enders, Leticia S F Pereira, Marcia F Mesko, Erico M M Flores, Cezar A Bizzi
Water removal is an essential step during crude oil production due to several problems such as increased transportation costs and high corrosion rate due to dissolved salts. Indirect low frequency ultrasonic energy (US), using baths, has been recently proposed as an effective alternative for crude oil demulsification. However, the reactor position during sonication and its influence on the demulsification efficiency for crude oil has not been evaluated. In this sense, the aim of this study was to develop an automated system based on an open source hardware for mapping the acoustic field distribution in an US bath operating at 35kHz using a hydrophone...
April 2, 2017: Ultrasonics Sonochemistry
https://www.readbyqxmd.com/read/28433393/potential-mobility-of-inorganic-nutrients-and-its-controls-at-the-sediment-water-interface-in-the-main-path-of-kuroshio-current-off-eastern-taiwan
#3
Fengxia Zhou, Xuelu Gao, Yong Zhang, Huamao Yuan, Jinming Song, Kai Liu, Bo Yang, Wen Zhuang
Surface sediments were collected from the main path of Kuroshio Current (KC) off eastern Taiwan (ETW), and laboratory incubation was conducted for the study of the nutrient exchange at the sediment-water interface. Exchange fluxes of NO3(-)-N, NO2(-)-N, NH4(+)-N, PO4(3-)-P and SiO3(2-)-Si under simulated site condition were -0.0866, 0.00146, 0.0634, -0.00812 and -0.181mmolm(-2)d(-1), respectively. This indicated that sediments in the studied area might act as a source of NO2(-)-N and NH4(+)-N and a sink of NO3(-)-N, PO4(3-)-P and SiO3(2-)-Si...
April 19, 2017: Marine Pollution Bulletin
https://www.readbyqxmd.com/read/28433208/elucidating-the-fate-of-a-mixed-toluene-dhm-methanol-and-i-propanol-plume-during-in-situ-bioremediation
#4
E Verardo, O Atteia, H Prommer
Organic pollutants such as solvents or petroleum products are widespread contaminants in soil and groundwater systems. In-situ bioremediation is a commonly used remediation technology to clean up the subsurface to eliminate the risks of toxic substances to reach potential receptors in surface waters or drinking water wells. This study discusses the development of a subsurface model to analyse the performance of an actively operating field-scale enhanced bioremediation scheme. The study site was affected by a mixed toluene, dihydromyrcenol (DHM), methanol, and i-propanol plume...
April 6, 2017: Journal of Contaminant Hydrology
https://www.readbyqxmd.com/read/28433148/mechanics-and-transport-phenomena-in-agarose-based-hydrogels-studied-by-compression-relaxation-tests
#5
Diego Caccavo, Sara Cascone, Serena Poto, Gaetano Lamberti, Anna Angela Barba
Hydrogels are widespread materials, used in several frontier fields, due to their peculiar behavior: they couple solvent mass transport to system mechanics, exhibiting viscoelastic and poroelastic characteristics. The full understanding of this behavior is crucial to correctly design such complex systems. In this study agarose gels has been investigated through experimental stress-relaxation tests and with the aid of a 3D poroviscoelastic model. At the investigated experimental conditions, the agarose gels samples show a prevalent viscoelastic behavior, revealing limited water transport and an increase of the stiffness as well as of the relaxation time along with the polymer concentration...
July 1, 2017: Carbohydrate Polymers
https://www.readbyqxmd.com/read/28432970/insights-into-key-factors-controlling-go-stability-in-natural-surface-waters
#6
Yang Gao, Xuemei Ren, Xiaoli Tan, Tasawar Hayat, Ahmed Alsaedi, Changlun Chen
The effects of pH, cations (Na(+), K(+), Mg(2+), Ca(2+) and Al(3+)), and anions (Cl(-), HCO3(-), HPO4(2-) and SO4(2-)) on graphene oxide (GO) stability were investigated to address the current limitations in the knowledge regarding the stability of GO in natural surface water and its underlying mechanism. The threshold values of cations that destabilize GO were obtained and affected by both pH and anions. By employing elemental mapping and studying the effects of polyacrylic acid (PAA) on GO sedimentation and the re-dispersion of GO aggregates, we find that the GO aggregates induced by Na(+) and K(+) via electric double layer suppression and by Ca(2+) and Al(3+) via strong complxing are difficult to re-disperse completely...
April 11, 2017: Journal of Hazardous Materials
https://www.readbyqxmd.com/read/28432152/exposure-to-seawater-increases-intestinal-motility-in-euryhaline-rainbow-trout-oncorhynchus-mykiss
#7
Jeroen Brijs, Grant W Hennig, Albin Gräns, Esmée Dekens, Michael Axelsson, Catharina Olsson
Upon exposure to seawater, euryhaline teleosts need to imbibe and desalinate seawater to allow for intestinal ion and water absorption, as this is essential for maintaining osmotic homeostasis. Despite the potential benefits of increased mixing and transport of imbibed water for increasing the efficiency of absorptive processes, the effect of water salinity on intestinal motility in teleosts remains unexplored. By qualitatively and quantitatively describing in vivo intestinal motility of euryhaline rainbow trout (Oncorhynchus mykiss), this study demonstrates that in freshwater, the most common motility pattern consisted of clusters of rhythmic, posteriorly propagating contractions that lasted ∼1-2 minutes followed by a period of quiescence lasting ∼4-5 minutes...
April 21, 2017: Journal of Experimental Biology
https://www.readbyqxmd.com/read/28431895/hemolymph-proteins-of-anopheles-gambiae-larvae-infected-by-escherichia-coli
#8
Xuesong He, Xiaolong Cao, Yan He, Krishna Bhattarai, Janet Rogers, Steve Hartson, Haobo Jiang
Anopheles gambiae is a major vector of human malaria and its immune system in part determines the fate of ingested parasites. Proteins, hemocytes and fat body in hemolymph are critical components of this system, mediating both humoral and cellular defenses. Here we assessed differences in the hemolymph proteomes of water- and E. coli-pricked mosquito larvae by a gel-LC-MS approach. Among the 1756 proteins identified, 603 contained a signal peptide but accounted for two-third of the total protein amount on the quantitative basis...
April 18, 2017: Developmental and Comparative Immunology
https://www.readbyqxmd.com/read/28431388/retention-and-transport-of-graphene-oxide-in-water-saturated-limestone-media
#9
Shunan Dong, Yuanyuan Sun, Bin Gao, Xiaoqing Shi, Hongxia Xu, Jianfeng Wu, Jichun Wu
In this work, column experiments were conducted to investigate the transport characteristics of graphene oxide (GO) nanoparticles in limestone media under various electrolytes, solution pH, and humic acid (HA) concentration conditions. In the limestone media, GO exhibited relatively low mobility with the mass recovery rate lower than 65.2%, even when solution ionic strength was low. The presence of HA enhanced its mobility. In addition, the presence of S(2-), a divalent anion, also promoted GO transport in limestone media compared to Cl(-) under similar ionic strength conditions through neutralizing more positive charge and thus diminishing the cation bridging...
April 17, 2017: Chemosphere
https://www.readbyqxmd.com/read/28431338/the-design-and-fabrication-of-beta-sensor-system-for-in-situ-diffusion-tests-in-mudstone-in-france
#10
Zhenhua Lin, Olivier Tillement, Marie-Genevieve Blanchin, Vivek Jindal, Agnès Vinsot, Romain V H Dagnelie, Virginie Blin, Yanick Lettry, Benoit Hautefeuille
Long term in situ diffusion experiments in the Callovian-Oxfordian mudstone (France) are designed in the context of nuclear waste management. β-emitters HTO and (36)Cl radiotracers are representative of neutral and anionic species in these experiments. Studies have been carried out to design an in situ beta monitoring system in order to quantify tracer migration in the rock pore water over time. The development, design and calibration of β-emitter radiation sensors were performed. An optimised geometry was calculated for the detection chamber of (36)Cl in solution (Ø×L=30×2mm(2)) via Monte-Carlo N-Particle transport simulation tools...
April 1, 2017: Applied Radiation and Isotopes
https://www.readbyqxmd.com/read/28431314/effect-of-metals-on-microcystin-abundance-and-environmental-fate
#11
Guofei Dai, Ningyan Peng, Jiayou Zhong, Ping Yang, Binchun Zou, Hui Chen, Qian Lou, Yuanyuan Fang, Wei Zhang
Metals can react with microcystin (MC), which is released from cyanobacterial blooms through various mechanisms; these reactions may mitigate the environmental and health risks of MCs but may also cause harm to aquatic ecosystems and humans. Several studies were conducted, including laboratory tests, ecological simulations, and a field investigation of Poyang Lake. The laboratory studies showed that Fe(3+), Cu(2+), and Pb(2+) stimulated MC photodegradation under high light intensity at the water-sediment interface, which reduced the MC accumulation in the sediment...
April 18, 2017: Environmental Pollution
https://www.readbyqxmd.com/read/28430444/molecular-structuring-and-percolation-transition-in-hydrated-sulfonated-poly-ether-ether-ketone-membranes
#12
Madhusmita Tripathy, Sunil Kumar P B, Abhijit P Deshpande
The extent of phase separation and water percolation in sulfonated membranes are the key to their performance in fuel cells. Toward this, the effect of hydration on the morphology and transport characteristics of sulfonated poly(ether ether ketone), sPEEK, membrane is investigated using atomistic molecular dynamics simulation at various hydration levels($\lambda$: number of water molecules per sulfonate group). The evolution of local morphology is investigated using structural correlations and minimum pair distances...
April 21, 2017: Journal of Physical Chemistry. B
https://www.readbyqxmd.com/read/28429776/global-distribution-of-particle-phase-state-in-atmospheric-secondary-organic-aerosols
#13
Manabu Shiraiwa, Ying Li, Alexandra P Tsimpidi, Vlassis A Karydis, Thomas Berkemeier, Spyros N Pandis, Jos Lelieveld, Thomas Koop, Ulrich Pöschl
Secondary organic aerosols (SOA) are a large source of uncertainty in our current understanding of climate change and air pollution. The phase state of SOA is important for quantifying their effects on climate and air quality, but its global distribution is poorly characterized. We developed a method to estimate glass transition temperatures based on the molar mass and molecular O:C ratio of SOA components, and we used the global chemistry climate model EMAC with the organic aerosol module ORACLE to predict the phase state of atmospheric SOA...
April 21, 2017: Nature Communications
https://www.readbyqxmd.com/read/28429634/migration-of-oligomers-from-pet-determination-of-diffusion-coefficients-and-comparison-of-experimental-versus-modelled-migration
#14
Maria Hoppe, Roberta Fornari, Pim de Voogt, Roland Franz
Polyethylene terephthalate is increasingly used as food contact material for example in containers for beverage such as bottles for soft drinks, mineral water, juices and beer. Mass transport of substances present in packaging materials into the packed food and beverages is monitored to verify the food law compliance of the materials. PET is known to contain or give rise to migrants that are oligomers derived from the polymeric material. Until now their actual migration potential has been investigated only poorly...
April 21, 2017: Food Additives & Contaminants. Part A, Chemistry, Analysis, Control, Exposure & Risk Assessment
https://www.readbyqxmd.com/read/28429410/photoelectroreduction-toward-chemical-building-blocks
#15
Fengjiao Chen, Wei Cui, Jie Zhang, Yeyun Wang, Junhua Zhou, Yongpan Hu, Yanguang Li, Shuit-Tong Lee
Conventional photoelectrochemical cells utilize solar energy to drive the chemical conversion of water or CO2 into useful chemical fuels. Such processes are confronted with general challenges, including the low intrinsic activities and inconvenient storage and transportation of their gaseous products. A photoelectrochemical approach is proposed to drive the reductive production of industrial building-block chemicals and demonstrate that succinic acid and glyoxylic acid can be readily synthesized on Si nanowire array photocathodes free of any cocatalyst and at room temperature...
April 21, 2017: Angewandte Chemie
https://www.readbyqxmd.com/read/28429011/drop-transport-and-positioning-on-lubricant-impregnated-surfaces
#16
Jian Hui Guan, Élfego Ruiz-Gutiérrez, Ben Bin Xu, David Wood, Glen McHale, Rodrigo Ledesma-Aguilar, Gary George Wells
We demonstrate the transport and positioning of water droplets on macro-patterned lubricant-impregnated surfaces. The macro-patterning produces menisci features in the impregnating liquid layer which interact with a droplet via a capillary mechanism similar to the Cheerios effect. These interactions control the droplet motion and positioning on an otherwise completely slippery surface. We present experimental results using a V-shape channel geometry as a model system. The interaction between deformations on the lubricant layer induced by the droplet and the underlying V-shape geometry leads to both local and global equilibrium positions for the droplet within the channel...
April 21, 2017: Soft Matter
https://www.readbyqxmd.com/read/28428820/regional-water-footprints-of-potential-biofuel-production-in-china
#17
Xiaomin Xie, Tingting Zhang, Liming Wang, Zhen Huang
BACKGROUND: Development of biofuels is considered as one of the important ways to replace conventional fossil energy and mitigate climate change. However, rapid increase of biofuel production could cause other environmental concerns in China such as water stress. This study is intended to evaluate the life-cycle water footprints (WF) of biofuels derived from several potential non-edible feedstocks including cassava, sweet sorghum, and Jatropha curcas in China. Different water footprint types including blue water, green water, and grey water are considered in this study...
2017: Biotechnology for Biofuels
https://www.readbyqxmd.com/read/28428443/mechanisms-of-pinometostat-epz-5676-treatment-emergent-resistance-in-mll-rearranged-leukemia
#18
Carly T Campbell, Jessica N Haladyna, David A Drubin, Ty M Thomson, Michael J Maria, Taylor Yamauchi, Nigel J Waters, Edward J Olhava, Roy M Pollock, Jesse J Smith, Robert A Copeland, Stephen J Blakemore, Kathrin M Bernt, Scott R Daigle
DOT1L is a protein methyltransferase involved in the development and maintenance of MLL-rearranged (MLL-r) leukemia through its ectopic methylation of histones associated with well characterized leukemic genes.  Pinometostat (EPZ-5676), a selective inhibitor of DOT1L, is in clinical development in relapsed/refractory acute leukemia patients harboring rearrangements of the MLL gene. The observation of responses and subsequent relapses in the adult trial treating MLL-r patients motivated preclinical investigations into potential mechanisms of pinometostat treatment emergent resistance (TER) in cell lines confirmed to have MLL-r...
April 20, 2017: Molecular Cancer Therapeutics
https://www.readbyqxmd.com/read/28427995/conditioned-taste-avoidance-conditioned-place-preference-and-hyperthermia-induced-by-the-second-generation-bath-salt-%C3%AE-pyrrolidinopentiophenone-%C3%AE-pvp
#19
Katharine H Nelson, Briana J Hempel, Matthew M Clasen, Kenner C Rice, Anthony L Riley
BACKGROUND: α-Pyrrolidinopentiophenone (α-PVP) has been reported to be rewarding in a variety of pre-clinical models. Given that a number of drugs of abuse have both rewarding and aversive effects, the balance of which influences addiction potential, the present study examined the aversive properties of α-PVP by assessing its ability to induce taste avoidance. This assessment was made in a combined taste avoidance/place conditioning design that also allowed an evaluation of the relationship between α-PVP's aversive and rewarding effects...
April 17, 2017: Pharmacology, Biochemistry, and Behavior
https://www.readbyqxmd.com/read/28426989/the-thermal-impact-of-subsurface-building-structures-on-urban-groundwater-resources-a-paradigmatic-example
#20
Jannis Epting, Stefan Scheidler, Annette Affolter, Paul Borer, Matthias H Mueller, Lukas Egli, Alejandro García-Gil, Peter Huggenberger
Shallow subsurface thermal regimes in urban areas are increasingly impacted by anthropogenic activities, which include infrastructure development like underground traffic lines as well as industrial and residential subsurface buildings. In combination with the progressive use of shallow geothermal energy systems, this results in the so-called subsurface urban heat island effect. This article emphasizes the importance of considering the thermal impact of subsurface structures, which commonly is underestimated due to missing information and of reliable subsurface temperature data...
April 17, 2017: Science of the Total Environment
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