Xiaoya Fan, Chaozhen Liu, Xun He, Zixiao Li, Luchao Yue, Wenxi Zhao, Jun Li, Yan Wang, Tingshuai Li, Yongsong Luo, Dongdong Zheng, Shengjun Sun, Qian Liu, Luming Li, Wei Chu, Feng Gong, Bo Tang, Yongchao Yao, Xuping Sun
Renewable electricity-powered nitrate/carbon dioxide co-reduction reaction toward urea production paves an attractive alternative to industrial urea processes and offers a clean on-site approach to closing the global nitrogen cycle. However, its large-scale implantation is severely impeded by challenging C-N coupling and requires electrocatalysts with high activity/selectivity. Here, cobalt-nanoparticles anchored on carbon nanosheet (Co NPs@C) is proposed as a catalyst electrode to boost yield and Faradaic efficiency (FE) toward urea electrosynthesis with enhanced C-N coupling...
April 2, 2024: Advanced Materials