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Disinfection byproduct

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https://www.readbyqxmd.com/read/28445816/disinfection-byproduct-formation-in-drinking-water-sources-a-case-study-of-yuqiao-reservoir
#1
Hongyan Zhai, Xizhen He, Yan Zhang, Tingting Du, Adeyemi S Adeleye, Yao Li
This study investigated the potential formation of disinfection byproducts (DBPs) during chlorination and chloramination of 20 water samples collected from different points of Yuqiao reservoir in Tianjin, China. The concentrations of dissolved organic matter and ammonia decreased downstream the reservoir, while the specific UV absorbance (SUVA: the ratio of UV254 to dissolved organic carbon) increased [from 0.67 L/(mg*m) upstream to 3.58 L/(mg*m) downstream]. The raw water quality played an important role in the formation of DBPs...
April 15, 2017: Chemosphere
https://www.readbyqxmd.com/read/28416302/effect-of-bacterial-biofilm-on-the-osteogenic-differentiation-of-stem-cells-of-apical-papilla
#2
Lakshmi Vishwanat, Rose Duong, Koyo Takimoto, Linda Phillips, Claudia O Espitia, Anibal Diogenes, Shivani B Ruparel, David Kolodrubetz, Nikita B Ruparel
INTRODUCTION: Although clinical success in regenerative endodontics is substantially high, histological success is limited to finding bone/cementum-like tissue instead of dentin within the canal space. The aims of this study were to investigate (1) the effect of bacterial biofilm on osteogenic gene expression in stem cells of the apical papilla (SCAP) and (2) the effect of bacterial antigens on the functional differentiation of SCAP into a mineralizing phenotype. METHODS: Using an ex vivo organotypic root canal model and an American Association of Endontists-recommended regenerative endodontic procedures, we evaluated SCAP differentiation in the presence and absence of an Enterococcus faecalis biofilm...
April 14, 2017: Journal of Endodontics
https://www.readbyqxmd.com/read/28391120/transformation-of-acesulfame-in-chlorination-kinetics-study-identification-of-byproducts-and-toxicity-assessment
#3
Adela Jing Li, Pengran Wu, Japhet Cheuk-Fung Law, Chi-Hang Chow, Cristina Postigo, Ying Guo, Kelvin Sze-Yin Leung
Acesulfame (ACE) is one of the most commonly used artificial sweeteners. Because it is not metabolized in the human gut, it reaches the aquatic environment unchanged. In the present study, the reactivity of ACE in free chlorine-containing water was investigated for the first time. The degradation of ACE was found to follow pseudo-first-order kinetics. The first-order rate increased with decreasing pH from 9.4 to 4.8 with estimated half-lives from 693 min to 2 min. Structural elucidation of the detected transformation products (TPs) was performed by ultra-high performance liquid chromatography coupled with quadrupole time-of-flight mass spectrometry...
March 28, 2017: Water Research
https://www.readbyqxmd.com/read/28377117/reductions-of-dissolved-organic-matter-and-disinfection-by-product-precursors-in-full-scale-wastewater-treatment-plants-in-winter
#4
Shuang Xue, Wujisiguleng Jin, Zhaohong Zhang, Hong Liu
The reductions of dissolved organic matter (DOM) and disinfection byproduct precursors in four full-scale wastewater treatment plants (WWTPs) (Liaoning Province, China) where different biological treatment processes were employed in winter were investigated. The total removal efficiencies of dissolved organic carbon (DOC), ultraviolet light at 254 nm (UV-254), trihalomethane formation potential (THMFP), and haloacetic acid formation potential (HAAFP) were in the range of 70.3-76.0%, 49.6-57.3%, 54.4-65.0%, and 53...
July 2017: Chemosphere
https://www.readbyqxmd.com/read/28334666/bio-refractory-dissolved-organic-matter-and-colorants-in-cassava-distillery-wastewater-characterization-coagulation-treatment-and-mechanisms
#5
Ming Zhang, Zhou Wang, Penghui Li, Hua Zhang, Li Xie
An important portion of organic matter and colorants still remain in the biologically treated distillery wastewater, leaving the dark brown and odorous downstream with the heavy loading of chemical oxygen demand and the potential of forming disinfection byproducts. However, those bio-recalcitrant colorants have not been clearly recognized. The current study investigated the features of the bio-refractory organic matter and colorants in a typical distillery effluent, cassava distillery wastewater; special attention was paid to their change and behaviors in the coagulation treatment following the bio-processes...
March 20, 2017: Chemosphere
https://www.readbyqxmd.com/read/28324709/improvement-of-virus-removal-using-ultrafiltration-membranes-modified-with-grafted-zwitterionic-polymer-hydrogels
#6
Ruiqing Lu, Chang Zhang, Maria Piatkovsky, Mathias Ulbricht, Moshe Herzberg, Thanh H Nguyen
Potable water reuse has been adopted by cities suffering water scarcity in recent years. The microbial safety in water reuse, especially with respect to pathogenic viruses, is still a concern for water consumers. Membrane filtration can achieve sufficient removal of pathogenic viruses without disinfection byproducts, but the required energy is intensive. In this study, we graft-polymerized zwitterionic SPP ([3-(methacryloylamino) propyl] dimethyl (3-sulfopropyl) ammonium hydroxide) on a 150 kDa ultrafiltration polyethersulfone membrane to achieve a significantly higher virus removal...
June 1, 2017: Water Research
https://www.readbyqxmd.com/read/28252454/ingested-nitrate-disinfection-by-products-and-kidney-cancer-risk-in-older-women
#7
Rena R Jones, Peter J Weyer, Curt T Dellavalle, Kim Robien, Kenneth P Cantor, Stuart Krasner, Laura E Beane Freeman, Mary H Ward
BACKGROUND: N-nitroso compounds formed endogenously after nitrate/nitrite ingestion are animal renal carcinogens. Previous epidemiologic studies of drinking water nitrate did not evaluate other potentially toxic water contaminants, including the suspected renal carcinogen chloroform. METHODS: In a cohort of postmenopausal women in Iowa (1986-2010), we used historical measurements to estimate long-term average concentrations of nitrate-nitrogen (NO3-N) and disinfection byproducts (DBP) in public water supplies...
March 1, 2017: Epidemiology
https://www.readbyqxmd.com/read/28248086/mass-spectrometry-identification-of-n-chlorinated-dipeptides-in-drinking-water
#8
Guang Huang, Ping Jiang, Xing-Fang Li
We report the identification of N-chlorinated dipeptides as chlorination products in drinking water using complementary high-resolution quadrupole time-of-flight (QTOF) and quadrupole ion-trap mass spectrometry techniques. First, three model dipeptides, tyrosylglycine (Tyr-Gly), tyrosylalanine (Tyr-Ala), and phenylalanylglycine (Phe-Gly), reacted with sodium hypochlorite, and these reaction solutions were analyzed by QTOF. N-Cl-Tyr-Gly, N,N-di-Cl-Tyr-Gly, N-Cl-Phe-Gly, N,N-di-Cl-Phe-Gly, N-Cl-Tyr-Ala, and N,N-di-Cl-Tyr-Ala were identified as the major products based on accurate masses, (35)Cl/(37)Cl isotopic patterns, and MS/MS spectra...
March 14, 2017: Analytical Chemistry
https://www.readbyqxmd.com/read/28235738/highly-efficient-and-environmentally-benign-as-iii-pre-oxidation-in-water-by-using-a-solid-redox-polymer
#9
Hongchao Li, Xiaolin Zhang, Mengfei Wu, Weiming Zhang, Lu Lv, Bingcai Pan
As(III) preoxidation to As(V) is usually a requisite step for its efficient removal from water. Traditional oxidants reacting with As(III) homogenously in water suffer from the excessive dosage as well as the possible formation of disinfection byproducts. Herein, we developed a heterogeneous oxidant, i.e., a solid redox polymer (DOX), by covalently binding chlorine to a commercially available cation-exchange resin, D001. As(III) pre-oxidation by DOX is independent upon the solution pH (6-8) and ionic strength (0-0...
May 2017: Chemosphere
https://www.readbyqxmd.com/read/28229949/predicting-reactivity-of-model-dom-compounds-towards-chlorine-with-mediated-electrochemical-oxidation
#10
Glen Andrew de Vera, Wolfgang Gernjak, Jelena Radjenovic
Chlorine demand of a water sample depends on the characteristics of dissolved organic matter (DOM). It is an important parameter for water utilities used to assess oxidant and/or disinfectant consumption of source waters during treatment and distribution. In this study, model compounds namely resorcinol, tannic acid, vanillin, cysteine, tyrosine, and tryptophan were used to represent the reactive moieties of complex DOM mixtures. The reactivity of these compounds was evaluated in terms of Cl2 demand and electron donating capacity (EDC)...
January 23, 2017: Water Research
https://www.readbyqxmd.com/read/28199792/removal-of-intermediate-aromatic-halogenated-dbps-by-activated-carbon-adsorption-a-new-approach-to-controlling-halogenated-dbps-in-chlorinated-drinking-water
#11
Jingyi Jiang, Xiangru Zhang, Xiaohu Zhu, Yu Li
During chlorine disinfection of drinking water, chlorine may react with natural organic matter (NOM) and bromide ion in raw water to generate halogenated disinfection byproducts (DBPs). To mitigate adverse effects from DBP exposure, granular activated carbon (GAC) adsorption has been considered as one of the best available technologies for removing NOM (DBP precursor) in drinking water treatment. Recently, we have found that many aromatic halogenated DBPs form in chlorination, and they act as intermediate DBPs to decompose and form commonly known DBPs including trihalomethanes and haloacetic acids...
February 28, 2017: Environmental Science & Technology
https://www.readbyqxmd.com/read/28196675/occurrence-of-brominated-disinfection-byproducts-in-the-air-and-water-of-chlorinated-seawater-swimming-pools
#12
Tarek Manasfi, Brice Temime-Roussel, Bruno Coulomb, Laurent Vassalo, Jean-Luc Boudenne
An undesirable consequence of disinfection is the formation of chemical contaminants known as disinfection byproducts (DBPs). Chronic exposure to DBPs has been linked to adverse health effects. The occurrence of DBPs in chlorinated pools filled with seawater (such as thalassotherapy pools and pools in spas) has received little attention so far. The present study evaluated the speciation and levels of disinfection byproducts in indoor swimming pools filled with seawater and treated with chlorine. Water and air samples were collected from three indoor swimming pools located in Southern France...
February 5, 2017: International Journal of Hygiene and Environmental Health
https://www.readbyqxmd.com/read/28187382/adsorption-of-natural-organic-matter-and-disinfection-byproduct-precursors-from-surface-water-onto-tio2-nanoparticles-ph-effects-isotherm-modelling-and-implications-for-using-tio2-for-drinking-water-treatment
#13
Stephanie L Gora, Susan A Andrews
Titanium dioxide is a photocatalyst that can remove organic contaminants of interest to the drinking water treatment industry, including natural organic matter (NOM) and disinfection byproduct (DBP) precursors. The photocatalytic reaction occurs in two steps: adsorption of the contaminant followed by degradation of the adsorbed contaminant upon irradiation with UV light. The second part of this process can lead to the formation of reactive intermediates and negative impacts on treated water quality, such as increased DBP formation potential (DBPfp)...
May 2017: Chemosphere
https://www.readbyqxmd.com/read/28174041/occurrence-origin-and-toxicity-of-disinfection-byproducts-in-chlorinated-swimming-pools-an-overview
#14
REVIEW
Tarek Manasfi, Bruno Coulomb, Jean-Luc Boudenne
Disinfection treatments are critical to conserve the microbiological quality of swimming pool water and to prevent water-borne infections. The formation of disinfection byproducts (DBPs) in swimming pools is an undesirable consequence resulting from reactions of disinfectants (e.g. chlorine) with organic and inorganic matter present in pool water, mainly brought by bathers. A considerable body of occurrence studies has identified several classes of DBPs in swimming pools with more than 100 compounds detected, mainly in chlorinated freshwater pools...
January 30, 2017: International Journal of Hygiene and Environmental Health
https://www.readbyqxmd.com/read/28171837/efficient-photoreductive-decomposition-of-n-nitrosodimethylamine-by-uv-iodide-process
#15
Zhuyu Sun, Chaojie Zhang, Xiaoyun Zhao, Jing Chen, Qi Zhou
N-nitrosodimethylamine (NDMA) has aroused extensive concern as a disinfection byproduct due to its high toxicity and elevated concentration levels in water sources. This study investigates the photoreductive decomposition of NDMA by UV/iodide process. The results showed that this process is an effective strategy for the treatment of NDMA with 99.2% NDMA removed within 10min. The depletion of NDMA by UV/iodide process obeyed pseudo-first-order kinetics with a rate constant (k1) of 0.60±0.03min(-1). Hydrated electrons (eaq(-)) generated by the UV irradiation of iodide were proven to play a critical role...
May 5, 2017: Journal of Hazardous Materials
https://www.readbyqxmd.com/read/28161516/identification-and-determination-of-disinfection-byproducts-in-chlorine-containing-household-cleansing-products
#16
Ho-Sang Shin, Hyun-Hee Lim
Seven halogenated volatile organic compounds (HVOCs) and two haloacetic acids were detected and quantified in 15 household products, including sodium hypochlorite, by gas chromatography-mass spectrometry (GC-MS). Chloroform was detected in a range of 0.2-30.2 mg kg(-1) in all products, and carbon tetrachloride was observed in 13 samples in a range of 0.05-352 mg kg(-1). Dichloroacetic acid and trichloroacetic acid were also detected up to 94 and 146 mg kg(-1) in household products. The estimated human exposures of chloroform, carbon tetrachloride, dichloroacetic acid and trichloroacetic acid were calculated to 0...
May 2017: Chemosphere
https://www.readbyqxmd.com/read/28153699/detection-formation-and-occurrence-of-13-new-polar-phenolic-chlorinated-and-brominated-disinfection-byproducts-in-drinking-water
#17
Yang Pan, Ying Wang, Aimin Li, Bin Xu, Qiming Xian, Chendong Shuang, Peng Shi, Qing Zhou
Recently, 13 new polar phenolic chlorinated and brominated disinfection byproducts (Cl- and Br-DBPs) were identified and quantified in simulated chlorinated drinking water by adopting product ion scan, precursor ion scan, and multiple reaction monitoring (MRM) analyses using ultra performance liquid chromatography/electrospray ionization-triple quadrupole mass spectrometry (UPLC/ESI-tqMS). The 13 new DBPs have been drawing increasing concern not only because they possess significantly higher growth inhibition, developmental toxicity, and chronic cytotoxicity than commonly known aliphatic DBPs, but also because they act as intermediate DBPs that can decompose to form the U...
January 24, 2017: Water Research
https://www.readbyqxmd.com/read/28118976/analysis-of-haloacetic-acids-bromate-and-dalapon-in-natural-waters-by-ion-chromatography-tandem-mass-spectrometry
#18
Shimin Wu, Tarun Anumol, Jay Gandhi, Shane A Snyder
The addition of oxidants for disinfecting water can lead to the formation of potentially carcinogenic compounds referred to as disinfection byproducts (DBPs). Haloacetic acids (HAAs) are one of the most widely detected DBPs in US water utilities and some of them are regulated by the US Environmental Protection Agency (USEPA). The present study developed a method to analyze all the compounds in the USEPA method 557 (nine HAAs, bromate and dalapon) plus four potentially more toxic iodinated HAAs in water by coupling ion chromatography with tandem mass spectrometry (IC-MS/MS)...
March 3, 2017: Journal of Chromatography. A
https://www.readbyqxmd.com/read/28110142/characteristics-of-water-obtained-by-dewatering-cyanobacteria-containing-sludge-formed-during-drinking-water-treatment-including-c-n-disinfection-byproduct-formation
#19
Hangzhou Xu, Haiyan Pei, Yan Jin, Hongdi Xiao, Chunxia Ma, Jiongming Sun, Hongmin Li
This is the first study to systematically investigate the characteristics of the water obtained by dewatering cyanobacteria-containing sludge generated in the drinking water treatment plant, including formation of C- and N-disinfection by-products (DBPs). Results showed that this 'dewatering water' (DW) had different properties when the sludge was stored at different times. The content of dissolved organic matter (DOM) and microcystins (MCs) in the DW were low when the sludge was treated or disposed of within 4 days; correspondingly, the C-, N-DBP production was also low...
January 13, 2017: Water Research
https://www.readbyqxmd.com/read/28098448/new-insights-into-trihalomethane-and-haloacetic-acid-formation-potentials-correlation-with-the-molecular-composition-of-natural-organic-matter-in-source-water
#20
Xin Wang, Haifeng Zhang, Yahe Zhang, Quan Shi, Juan Wang, Jianwei Yu, Min Yang
Natural organic matter (NOM) represents the major source of precursors for disinfection byproducts (DBPs), such as trihalomethanes (THMs) and haloacetic acids (HAAs), formed during disinfection of drinking water, but the molecular composition and reactivity of NOM remain not well understood. In this study, electrospray ionization coupled to Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS) was used to characterize the molecular composition of NOM of 20 source waters taken across China for the purpose of determining the major precursors of THMs and HAAs at molecular level...
February 2, 2017: Environmental Science & Technology
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