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https://www.readbyqxmd.com/read/28088150/optimal-orientation-of-an-asymmetric-top-molecule-with-terahertz-pulses
#1
L H Coudert
Terahertz pulses effects are investigated in an asymmetric top C2v molecule using numerical simulations. The average value of the direction cosine ΦZx is computed solving the time dependent Schrödinger equation for several types of pulses. The H2S molecule taken as a test case is first subject to two short terahertz pulses with a duration smaller than 5 ps, an identical maximum value of the electric field of 2 MV/cm, but a different shape. The thermal average ⟨⟨ΦZx⟩⟩ is calculated for several temperatures, and non-periodic time variations are found even for the lowest temperature...
January 14, 2017: Journal of Chemical Physics
https://www.readbyqxmd.com/read/28088149/collective-excitations-in-liquid-dimethyl-sulfoxide-dmso-fir-spectrum-low-frequency-vibrational-density-of-states-and-ultrafast-dipolar-solvation-dynamics
#2
Milan K Hazra, Biman Bagchi
Valuable dynamical and structural information about neat liquid DMSO at ambient conditions can be obtained through a study of low frequency vibrations in the far infrared (FIR), that is, terahertz regime. For DMSO, collective excitations as well as single molecule stretches and bends have been measured by different kinds of experiments such as OHD-RIKES and terahertz spectroscopy. In the present work, we investigate the intermolecular vibrational spectrum of DMSO through three different computational techniques namely (i) the far-infrared spectrum obtained through the Fourier transform of total dipole moment auto-time correlation function, (ii) from the Fourier transform of the translational and angular velocity time autocorrelation functions, and (iii) a quenched normal mode analysis of the parent liquid at 300 K...
January 14, 2017: Journal of Chemical Physics
https://www.readbyqxmd.com/read/28081098/generation-of-terahertz-optical-beating-from-a-simultaneously-self-mode-locked-nd-yag-laser-at-1064-and-1123%C3%A2-%C3%A2-nm
#3
C L Sung, C Y Lee, C C Chang, H C Liang, Y F Chen
The reflectivity of the output coupler is designed to achieve the synchronously self-mode-locked operation at 1064 and 1123 nm in a diode-end-pumped Nd:YAG laser. Numerical analyses are performed to confirm that the designed output coupler can lead the emission lines to be predominant at 1064 and 1123 nm. Moreover, the crossover of the threshold pump powers for the 1064 and 1123 nm emission lines can be exploited to obtain the single central wavelength of 1064 nm or the single central wavelength of 1123 nm or, simultaneously, dual-central-wavelength self-mode-locked operation by finely adjusting the cavity alignment...
January 15, 2017: Optics Letters
https://www.readbyqxmd.com/read/28081067/guiding-terahertz-orbital-angular-momentum-beams-in-multimode-kagome-hollow-core-fibers
#4
Haisu Li, Guobin Ren, Bofeng Zhu, Yixiao Gao, Bin Yin, Jing Wang, Shuisheng Jian
We explore terahertz (THz) orbital angular momentum (OAM) modes supported in multimode Kagome hollow-core fibers. Numerical models are adopted to characterize the effective indices and confinement losses of vector modes over 0.2-0.9 THz, where two low-loss transmission windows are observed. Linearly combining the vector modes, THz OAM states can be generated. Covering a broad bandwidth of 0.25 THz, the purity values of OAM modes are beyond 0.9. Using numerical simulations, the hollow-core THz fibers with one and two rings of Kagome structures are also comparably investigated...
January 15, 2017: Optics Letters
https://www.readbyqxmd.com/read/28071764/aligned-copper-nanorod-arrays-for-highly-efficient-generation-of-intense-ultra-broadband-thz-pulses
#5
S Mondal, Q Wei, W J Ding, H A Hafez, M A Fareed, A Laramée, X Ropagnol, G Zhang, S Sun, Z M Sheng, J Zhang, T Ozaki
We demonstrate an intense broadband terahertz (THz) source based on the interaction of relativistic-intensity femtosecond lasers with aligned copper nanorod array targets. For copper nanorod targets with a length of 5 μm, a maximum 13.8 times enhancement in the THz pulse energy (in ≤20 THz spectral range) is measured as compared to that with a thick plane copper target under the same laser conditions. A further increase in the nanorod length leads to a decrease in the THz pulse energy at medium frequencies (≤20 THz) and increase of the electromagnetic pulse energy in the high-frequency range (from 20-200 THz)...
January 10, 2017: Scientific Reports
https://www.readbyqxmd.com/read/28071681/increased-impedance-near-cut-off-in-plasma-like-media-leading-to-emission-of-high-power-narrow-bandwidth-radiation
#6
M S Hur, B Ersfeld, A Noble, H Suk, D A Jaroszynski
Ultra-intense, narrow-bandwidth, electromagnetic pulses have become important tools for exploring the characteristics of matter. Modern tuneable high-power light sources, such as free-electron lasers and vacuum tubes, rely on bunching of relativistic or near-relativistic electrons in vacuum. Here we present a fundamentally different method for producing narrow-bandwidth radiation from a broad spectral bandwidth current source, which takes advantage of the inflated radiation impedance close to cut-off in a medium with a plasma-like permittivity...
January 10, 2017: Scientific Reports
https://www.readbyqxmd.com/read/28070085/application-of-terahertz-time-domain-spectroscopy-in-detecting-gaps-with-different-widths
#7
Rima Bao, Zhikui Wu, Fang Wang, Xinyang Miao, Chengjing Feng
The characterization of fractures is of vital importance for studies in many industries. In the present work, we used terahertz reflection measurements to identify simulated gaps of different widths that resemble fractures. The time interval between pulses (Δt) was proportional to the distance between the interfaces. In addition, fast Fourier transform (FFT) corresponding to the waveforms was also employed to distinguish the gaps. The widths in frequency were found to be inversely proportional to that of the gaps...
2017: Analytical Sciences: the International Journal of the Japan Society for Analytical Chemistry
https://www.readbyqxmd.com/read/28067289/optical-and-thz-investigations-of-mid-ir-materials-exposed-to-alpha-particle-irradiation
#8
Dan Sporea, Laura Mihai, Adelina Sporea, Ion Vâţã
The paper is the first comprehensive study on alpha particle irradiation effects on four mid-IR materials: CaF2, BaF2, Al2O3 (sapphire) and ZnSe. The measurements of the optical spectral transmittance, spectral diffuse reflectance, radioluminescent emission, terahertz (THz) spectral response, transmittance, absorbance, refractive index, real and imaginary parts of the dielectric constant and THz imaging are used as complementary investigations to evaluate these effects. The simulations were run to estimate: (i) the penetration depth, (ii) the scattering of alpha particle beam, (iii) the amount of material affected by this interaction, and (iv) the number of vacancies produced by the radiation exposure for each type of material...
January 9, 2017: Scientific Reports
https://www.readbyqxmd.com/read/28067205/tunable-terahertz-reflection-of-graphene-via-ionic-liquid-gating
#9
Yang Wu, Xuepeng Qiu, Hongwei Liu, Jingbo Liu, Yan Chen, Lin Ke, Hyunsoo Yang
We report a highly efficient tunable THz reflector in graphene. By applying a small gate voltage (up to �� 3 V), the reflectance of graphene is modulated from a minimum of 0.79% to a maximum of 33.4% using graphene/ionic liquid structures at room temperature, and the reflection tuning is uniform within a wide spectral range (0.1 ��� 1.5 THz). Our observation is explained by the Drude model, which describes the THz wave-induced intraband transition in graphene. This tunable reflectance of graphene may contribute to broadband THz mirrors, deformable THz mirrors, variable THz beam splitters and other optical components...
January 9, 2017: Nanotechnology
https://www.readbyqxmd.com/read/28063427/hydrogen-bond-breaking-dynamics-in-the-water-pentamer-terahertz-vrt-spectroscopy-of-a-20-%C3%AE-m-libration
#10
William T S Cole, Raymond S Fellers, Mark R Viant, Richard J Saykally
Hydrogen bonds in solid and liquid water are formed and broken via librational vibrations, hence characterizing the details of these motions is vital to understanding these important dynamics. Here we report the measurement and assignment of 875 transitions comprising 6 subbands originating from out-of-plane librational transitions of the water pentamer-d10 near 512 cm(-1). The precisely measured (ca. 1 ppm) transitions reveal bifurcation splittings of ∼1884 MHz, a ∼4000× enhancement over ground state splittings and 100× greater than predicted by theory...
January 7, 2017: Journal of Chemical Physics
https://www.readbyqxmd.com/read/28059385/investigation-of-hollow-cylindrical-metal-terahertz-waveguides-suitable-for-cryogenic-environments
#11
R Wallis, R Degl Innocenti, D S Jessop, O Mitrofanov, C M Bledt, J E Melzer, J A Harrington, H E Beere, D A Ritchie
The field of terahertz (THz) waveguides continues to grow rapidly, with many being tailored to suit the specific demands of a particular final application. Here, we explore waveguides capable of enabling efficient and accurate power delivery within cryogenic environments (< 4 K). The performance of extruded hollow cylindrical metal waveguides made of un-annealed and annealed copper, as well as stainless steel, have been investigated for bore diameters between 1.75 - 4.6 mm, and at frequencies of 2.0, 2.85 and 3...
December 26, 2016: Optics Express
https://www.readbyqxmd.com/read/28059347/ultra-compact-injection-terahertz-laser-using-the-resonant-inter-layer-radiative-transitions-in-multi-graphene-layer-structure
#12
Alexander A Dubinov, Andrey Bylinkin, Vladimir Ya Aleshkin, Victor Ryzhii, Taiichi Otsuji, Dmitry Svintsov
The optimization of laser resonators represents a crucial issue for the design of tera-hertz semiconductor lasers with high gain and low absorption loss. In this paper, we put forward and optimize the surface plasmonic metal waveguide geometry for the recently proposed tera-hertz injection laser based on resonant radiative transitions between tunnel-coupled graphene layers. We find an optimal number of active graphene layer pairs corresponding to the maximum net modal gain. The maximum gain increases with frequency and can be as large as ∼ 500 cm<sup>-1</sup> at 8 THz, while the threshold length of laser resonator can be as small as ∼ 50 μm...
December 26, 2016: Optics Express
https://www.readbyqxmd.com/read/28059309/single-shot-terahertz-time-domain-spectroscopy-in-pulsed-high-magnetic-fields
#13
G Timothy Noe, Ikufumi Katayama, Fumiya Katsutani, James J Allred, Jeffrey A Horowitz, David M Sullivan, Qi Zhang, Fumiya Sekiguchi, Gary L Woods, Matthias C Hoffmann, Hiroyuki Nojiri, Jun Takeda, Junichiro Kono
We have developed a single-shot terahertz time-domain spectrometer to perform optical-pump/terahertz-probe experiments in pulsed, high magnetic fields up to 30 T. The single-shot detection scheme for measuring a terahertz waveform incorporates a reflective echelon to create time-delayed beamlets across the intensity profile of the optical gate beam before it spatially and temporally overlaps with the terahertz radiation in a ZnTe detection crystal. After imaging the gate beam onto a camera, we can retrieve the terahertz time-domain waveform by analyzing the resulting image...
December 26, 2016: Optics Express
https://www.readbyqxmd.com/read/28059288/tunable-resolution-terahertz-dual-frequency-comb-spectrometer
#14
Francisco S Vieira, Flavio C Cruz, David F Plusquellic, Scott A Diddams
Terahertz dual frequency comb spectroscopy (THz-DFCS) yields high spectral resolution without compromising bandwidth. Nonetheless, the resolution of THz-DFCS is usually limited by the laser repetition rate, which is typically between 80 MHz and 1 GHz. In this paper, we demonstrate a new method to achieve sub-repetition rate resolution in THz-DFCS by adaptively modifying the effective laser repetition rate using integrated Mach-Zehnder electro-optic modulators (MZ-EOMs). Our results demonstrate that it is possible to improve the 100 MHz resolution of a terahertz frequency comb by at least 20x (down to 5 MHz) across the terahertz spectrum without compromising the average output power, and to a large extent, its bandwidth...
December 26, 2016: Optics Express
https://www.readbyqxmd.com/read/28059253/coplanar-waveguide-wideband-band-stop-filter-based-on-localized-spoof-surface-plasmons
#15
Zhuo Li, Jia Xu, Chen Chen, Yunhe Sun, Bingzheng Xu, Liangliang Liu, Changqing Gu
In this work, a wideband band-stop plasmonic filter based on localized spoof surface plasmons is reported, which consists of a coplanar waveguide (CPW) and an ultra-thin periodic corrugated metallic strip with defect units at the back of the substrate. Defect units are used to localize the transmission energy along the CPW. Each defect unit can introduce a narrow stop band, and a series of defect units is judiciously designed to form a broadband CPW band-stop filter. The center frequency and bandwidth of the filter can be tuned by the heights and numbers of the defect units...
December 20, 2016: Applied Optics
https://www.readbyqxmd.com/read/28059237/noncontact-detection-of-teflon-inclusions-in-glass-fiber-reinforced-polymer-composites-using-terahertz-imaging
#16
Jin Zhang, Jie Wang, Xiaohui Han, Hong-Liang Cui, Changcheng Shi, Jinbo Zhang, Yan Shen
We employed terahertz (THz) time-domain spectroscopy (TDS) imaging technology, a new nondestructive testing method, to detect the inclusions of glass-fiber-reinforced polymer (GFRP) composites. The refractive index and absorption coefficient of two types of GFRP composites (epoxy GFRP composites and polyester GFRP composites) were first extracted, and GFRP composites with Teflon inclusions were examined, including an epoxy GFRP solid panel with a smaller Teflon inclusion hidden behind a larger Teflon inclusion, and polyester GFRP solid panels with Teflon inclusions of various sizes, at different depths...
December 20, 2016: Applied Optics
https://www.readbyqxmd.com/read/28059173/geometric-phase-shaping-of-terahertz-vortex-beams
#17
Amalya Minasyan, Clément Trovato, Jérôme Degert, Eric Freysz, Etienne Brasselet, Emmanuel Abraham
We propose a topological beam-shaping strategy of terahertz (THz) beams using geometric phase elements made of space-variant birefringent slabs. Quasi-monochromatic THz vortex beams are produced and characterized both in amplitude and phase from the reconstructed real-time two-dimensional imaging of the electric field. Nonseparable superpositions of such vortex beams are also obtained and characterized by two-dimensional polarimetric analysis. These results emphasize the versatility of the spin-orbit electromagnetic toolbox to prepare on-demand structured light endowed with polarization-controlled orbital angular momentum content in the THz domain, which should find many uses in future THz technologies...
January 1, 2017: Optics Letters
https://www.readbyqxmd.com/read/28050908/crystallization-kinetics-of-lead-halide-perovskite-film-monitored-by-in-situ-terahertz-spectroscopy
#18
S J Park, A R Kim, J T Hong, J Y Park, S Lee, Y H Ahn
Vibrational modes in the terahertz (THz) frequency range are good indicators of lead halide perovskite's crystallization phase. We performed real-time THz spectroscopy to monitor the crystallization kinetics in the perovskite films. First, THz absorptance was measured while the perovskite film was annealed at different temperatures. By analyzing the Avrami exponent, we observed an abrupt dimensionality switch (from 1D to 2D) with increasing temperature starting at approximately 90 °C. We also monitored the laser-induced crystallinity enhancement of the preannealed perovskite film...
January 5, 2017: Journal of Physical Chemistry Letters
https://www.readbyqxmd.com/read/28039969/classical-investigation-of-long-range-coherence-in-biological-systems
#19
Jordane Preto
Almost five decades ago, H. Fröhlich [H. Fröhlich, "Long-range coherence and energy storage in biological systems," Int. J. Quantum Chem. 2(5), 641-649 (1968)] reported, on a theoretical basis, that the excitation of quantum modes of vibration in contact with a thermal reservoir may lead to steady states, where under high enough rate of energy supply, only specific low-frequency modes of vibration are strongly excited. This nonlinear phenomenon was predicted to occur in biomolecular systems, which are known to exhibit complex vibrational spectral properties, especially in the terahertz frequency domain...
December 2016: Chaos
https://www.readbyqxmd.com/read/28019076/theoretical-evaluation-of-terahertz-sources-generating-from-infrared-nonlinear-optical-materials-snga4q7-q-s-se
#20
Wen-Dan Cheng, Chen-Sheng Lin, Hao Zhang, Yi-Zhi Huang, Guo-Liang Chai
We have theoretically evaluated the integrate knowledge, which contribute to conversion efficiency, including the phonon, photon and electron properties of infrared nonlinear optical materials SnGa4Q7 (Q = S, Se) being as terahertz (THz) sources. Specially, we have developed a new formula to calculate susceptibility of difference frequency generation (DFG) optical process. By the characteristics of materials-self properties in the THz region, we find that a larger nonlinear susceptibility or a large figure of merit will result in a large efficiency of THz source by the comparisons between the findings of SnGa4Se7 and SnGa4S7 under the same experimental conditions, and the THz absorption will reduce the efficiency of THz source for the two materials of SnGa4Q7 (Q = S, Se)...
December 25, 2016: Chemphyschem: a European Journal of Chemical Physics and Physical Chemistry
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