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https://www.readbyqxmd.com/read/28731772/publisher-s-note-infrared-topological-plasmons-in-graphene-phys-rev-lett-118-245301-2017
#1
Dafei Jin, Thomas Christensen, Marin Soljac Ić, Nicholas X Fang, Ling Lu, Xiang Zhang
This corrects the article DOI: 10.1103/PhysRevLett.118.245301.
July 7, 2017: Physical Review Letters
https://www.readbyqxmd.com/read/28731769/first-principles-prediction-of-spin-polarized-multiple-dirac-rings-in-manganese-fluoride
#2
Yalong Jiao, Fengxian Ma, Chunmei Zhang, John Bell, Stefano Sanvito, Aijun Du
Spin-polarized materials with Dirac features have sparked great scientific interest due to their potential applications in spintronics. But such a type of structure is very rare and none has been fabricated. Here, we investigate the already experimentally synthesized manganese fluoride (MnF_{3}) as a novel spin-polarized Dirac material by using first-principles calculations. MnF_{3} exhibits multiple Dirac cones in one spin orientation, while it behaves like a large gap semiconductor in the other spin channel...
July 7, 2017: Physical Review Letters
https://www.readbyqxmd.com/read/28731700/nanomanipulation-of-individual-dna-molecules-covered-by-single-layered-reduced-graphene-oxide-sheets-on-a-solid-substrate
#3
Ying Wang, Yue Shen, Bin Li, Shuo Wang, Jinjin Zhang, Yi Zhang, Jun Hu
Nanomanipulation of single DNA molecules has great potential in fundamental genetic research and clinical analysis, and is a good model system for studying the interfacial effects on physiochemical processes, which occur when manipulating the linear DNA molecules with an atomic force microscope (AFM) tip. Here, we demonstrate that AFM nanomanipulation can be carried out on DNA molecules covered by a single-layered reduced graphene oxide sheet. Nanomanipulation, which includes cutting, pushing, and sweeping operations, specific to the covered DNA molecules can be achieved in a well-controlled manner using AFM in the PeakForce Quantitative Nano-Mechanics mode...
July 21, 2017: Journal of Physical Chemistry. B
https://www.readbyqxmd.com/read/28731426/ultrahigh-electrical-and-thermal-conductive-hydroxylated-graphene-based-flexible-carbon-film
#4
Jiheng Ding, Obaid Ur Rahman, Hongran Zhao, Wanjun Peng, Huimin Dou, Hao Chen, Haibin Yu
Graphene based films are widely used in the electronics industry. Present work report surface hydroxylated graphene sheets (HGS) from natural graphite by a rapid and efficient molten hydroxide-assisted exfoliated technique. This method enable preparation of a flexible carbon film from exfoliated graphene with extraodinary production yield (~100%), high electrical (11.5×104 S. m-1) and thermal conductivity (1842 W m-1K -1) withbetter dispersion concentration (~10.0 mg mL-1). As a result, this method is expected to applied for the preparation of large-scale, high-quality and low-cost electrical and thermal conductive graphene based material...
July 21, 2017: Nanotechnology
https://www.readbyqxmd.com/read/28731318/ultrafast-ionic-liquid-assisted-microwave-synthesis-of-sno-microflowers-and-their-superior-sodium-ion-storage-performance
#5
Bingsheng Qin, Huang Zhang, Thomas Diemant, Dorin Geiger, Rinaldo Raccichini, R Jürgen Behm, Ute Kaiser, Alberto Varzi, Stefano Passerini
Tin oxide (SnO) is considered one of the most promising metal oxides for utilization as anode material in sodium ion batteries (SIBs), due to its ease of synthesis, high specific gravimetric capacity and satisfactory cycling performance. However, to aim at practical applications, the coulombic efficiency during cycling needs to be further improved, which requires a deeper knowledge of its working mechanism. Here, a microflower-shaped SnO material is synthesized by means of an ultrafast ionic liquid-assisted microwave method...
July 21, 2017: ACS Applied Materials & Interfaces
https://www.readbyqxmd.com/read/28731283/covalent-functionalization-of-graphene-by-nucleophilic-addition-reaction-synthesis-and-optical-limiting-property
#6
Xiujuan Xu, Peiying Li, Lei Zhang, Xuejian Liu, Hao-Li Zhang, Qingzhao Shi, Baojiang He, Wenjuan Zhang, Zhan Qu, Pu Liu
Covalent functionalization of reduced graphene oxide (rGO) was prepared by conjugated polymers with different monomers, using nucleophilic addition reaction between rGO and nitrogen anions. Three conjugated polymers containing tetraphenylethylene, carbazole and phenyl groups were used, due to the π-π interaction and "polymer wrapping" effect, the dispersion stability of rGO was improved. Even the reacting site in polymers were same to each other, there were great differences in the reactivity of the polymers, the dispersion stability of the resultant composites, and also the OL performances of the resultant composites...
July 21, 2017: Chemistry, An Asian Journal
https://www.readbyqxmd.com/read/28731224/extremely-low-density-and-super-compressible-graphene-cellular-materials
#7
Ling Qiu, Bing Huang, Zijun He, Yuanyuan Wang, Zhiming Tian, Jefferson Zhe Liu, Kun Wang, Jingchao Song, Thomas R Gengenbach, Dan Li
Development of extremely low density graphene elastomer (GE) holds the potential to enable new properties that traditional cellular materials cannot offer, which are promising for a range of emerging applications, ranging from flexible electronics to multifunctional scaffolds. However, existing graphene foams with extremely low density are generally found to have very poor mechanical resilience. It is scientifically intriguing but remains unresolved whether and how the density limit of this class of cellular materials can be further pushed down while their mechanical resilience is being retained...
July 21, 2017: Advanced Materials
https://www.readbyqxmd.com/read/28731077/high-performance-adsorption-and-separation-of-anionic-dyes-in-water-using-a-chemically-stable-graphene-like-metal-organic-framework
#8
Jun-Jiao Li, Chong-Chen Wang, Hui-Fen Fu, Jing-Rui Cui, Peng Xu, Jie Guo, Jian-Rong Li
A highly stable graphene-like metal-organic framework (BUC-17) was prepared and used as an adsorbent to carry out the adsorption of anionic dyes from simulated wastewater, which exhibited excellent adsorption performance, particularly towards Congo red (CR) up to 4923.7 mg g(-1) at room temperature. It was used to fix a SPE column to conduct rapid separation of anionic dyes from an organic dye matrix. A related mechanism was also proposed.
July 21, 2017: Dalton Transactions: An International Journal of Inorganic Chemistry
https://www.readbyqxmd.com/read/28730821/efficient-carrier-to-exciton-conversion-in-field-emission-tunnel-diodes-based-on-mis-type-van-der-waals-heterostack
#9
Shunfeng Wang, Junyong Wang, Weijie Zhao, Francesco Giustiniano, Leiqiang Chu, Ivan Verzhbitskiy, Justin Zhou Yong, Goki Eda
We report on efficient carrier-to-exciton conversion and planer electroluminescence from tunnel diodes based on a metal-insulator-semiconductor van der Waals heterostack consisting of few-layer graphene (FLG), hexagonal boron nitride (hBN), and monolayer tungsten disulfide (WS2). These devices exhibit excitonic electroluminescence with extremely low threshold current density of a few pA∙μm-2, which is several orders of magnitude lower compared to the previously reported values for the best planar EL devices...
July 21, 2017: Nano Letters
https://www.readbyqxmd.com/read/28730803/3d-graphene-foam-filled-elastomer-composites-with-high-thermal-and-mechanical-properties
#10
Haoming Fang, Yunhong Zhao, Yafei Zhang, Yanjuan Ren, Shulin Bai
In order to meet the increasing demands for effective heat management of electronic devices, graphene based polymeric composite is considered to be one of the candidate materials due to the ultrahigh thermal conductivity of graphene. However, poor graphene dispersion, low quality of exfoliated graphene and strong phonon scattering at graphene/matrix interface restrict the heat dissipation ability of graphene filled composites. Here, a facile and versatile approach to bond graphene foam (GF) with polydimethylsiloxane (PDMS) is proposed and the corresponding composite with considerable improvement of thermal conductivity and insulativity is fabricated...
July 21, 2017: ACS Applied Materials & Interfaces
https://www.readbyqxmd.com/read/28730702/high-performance-graphene-ni2-p-hybrid-anodes-for-lithium-and-sodium-storage-through-3d-yolk-shell-like-nanostructural-design
#11
Chao Wu, Peter Kopold, Peter A van Aken, Joachim Maier, Yan Yu
No abstract text is available yet for this article.
July 2017: Advanced Materials
https://www.readbyqxmd.com/read/28730306/disposable-electrochemical-immunosensor-for-brettanomyces-bruxellensis-based-on-nanogold-reduced-graphene-oxide-hybrid-nanomaterial
#12
Boryana Borisova, María L Villalonga, María Arévalo-Villena, Abderrahmane Boujakhrout, Alfredo Sánchez, Concepción Parrado, José M Pingarrón, Ana Briones-Pérez, Reynaldo Villalonga
The assembly of a novel disposable amperometric immunosensor for the detection of the red wine spoilage yeast Brettanomyces bruxellensis is reported. The nanostructured sensing interface was prepared by first coating carbon screen printed electrodes with a gold nanoparticles-reduced graphene oxide hybrid nanomaterial, which was then modified with 3-mercaptopropionic acid to further immobilize specific antibodies for B. bruxellensis via a carbodiimide-coupling reaction. The functionalized electrode allowed the amperometric detection of B...
July 20, 2017: Analytical and Bioanalytical Chemistry
https://www.readbyqxmd.com/read/28730215/energetics-and-diffusion-of-liquid-water-and-hydrated-ions-through-nanopores-in-graphene-ab-initio-molecular-dynamics-simulation
#13
Raúl Guerrero-Avilés, Walter Orellana
The energetics and diffusion of water molecules and hydrated ions (Na(+), Cl(-)) passing through nanopores in graphene are addressed by dispersion-corrected density functional theory calculations and ab initio molecular dynamics (MD) simulations. Pores of about 0.8 nm in diameter with different pore-edge passivations, with (H) and (O, H) atoms, were considered. Our MD simulations show a water flux through the hydroxylated pores of about one H2O molecule every three picoseconds, in close agreement with recent experiments that estimated a water flux of three molecules per picosecond through pores of ∼1 nm...
July 21, 2017: Physical Chemistry Chemical Physics: PCCP
https://www.readbyqxmd.com/read/28728900/ultra-sensitive-aptasensor-based-on-a-gqd-nanocomposite-for-detection-of-hepatitis-c-virus-core-antigen
#14
Kazhal Ghanbari, Mahmoud Roushani, Azadeh Azadbakht
In the present study, by using the aptamer proximity binding assay strategy, a novel electrochemical aptasensor is described for ultrasensitive detection of hepatitis C virus (HCV) core antigen. The immobilization surface is prepared by the modification of a glassy carbon electrode (GCE) with a graphene quantum dots (GQD). GQD were introduced as a novel and suitable substrate for aptamers through π-π stacking interactions, the richness of hydrophilic edges as well as hydrophobic plane in GQD which enhances the aptamer absorption on the electrode surface...
July 17, 2017: Analytical Biochemistry
https://www.readbyqxmd.com/read/28728125/assessment-and-prediction-of-joint-algal-toxicity-of-binary-mixtures-of-graphene-and-ionic-liquids
#15
Zhuang Wang, Fan Zhang, Se Wang, Willie J G M Peijnenburg
Graphene and ionic liquids (ILs) released into the environment will interact with each other. So far however, the risks associated with the concurrent exposure of biota to graphene and ILs in the environment have received little attention. The research reported here focused on observing and predicting the joint toxicity effects in the green alga Scenedesmus obliquus exposed to binary mixtures of intrinsic graphene (iG)/graphene oxide (GO) and five ILs of varying anionic and cationic types. The isolated ILs in the binary mixtures were the main contributors to toxicity...
July 8, 2017: Chemosphere
https://www.readbyqxmd.com/read/28728032/tunable-fluorescence-quenching-near-the-graphene-aqueous-interface
#16
Aaron W Chen, Alejandro L Briseno, Maria M Santore
With increased interest in graphene-based sensors for biomolecules and other targets, we investigated the impact of ionic strength on the steady-state emissions from fluorescein labels on proteins adsorbing on pristine CVD (chemical vapor deposited)-graphene on a silica support. Using the model system of fluorescein-tagged fibrinogen we demonstrated that, for fluorescein tags on adsorbed fibrinogen, emission intensity was very sensitive to the salt concentration. This behavior was not seen for fluorescein-tagged fibrinogen in solution...
July 6, 2017: Journal of Colloid and Interface Science
https://www.readbyqxmd.com/read/28728009/bridged-rebar-graphene-functionalized-aptasensor-for-pathogenic-e-coli-o78-k80-h11-detection
#17
Harmanjit Kaur, Munish Shorie, Manju Sharma, Ashok K Ganguli, Priyanka Sabherwal
We report a novel fabrication method of functionalised Bridged Rebar Graphene (BRG) onto newly designed nanostructured aptasensor for label free impedimetric sensing of pathogenic bacteria E. coli O78:K80:H11. The chemical facilitated unscrolling of MWCNT and subsequent bridging with terephthalaldehyde (TPA) to form 3D-hierarchical BRG nanoconstruct exhibited synergistic effect by combining enhanced electrical properties and facile chemical functionality for stable bio-interface. The bacteria-DNA interactions were captured on BRG nanostructured electrode by using specific anti-E...
July 5, 2017: Biosensors & Bioelectronics
https://www.readbyqxmd.com/read/28728007/direct-immune-detection-of-cortisol-by-chemiresistor-graphene-oxide-sensor
#18
Yo-Han Kim, Kyungmin Lee, Hunsang Jung, Hee Kyung Kang, Jihoon Jo, In-Kyu Park, Hyun Ho Lee
In this study, a biosensor to detect a stress biomarker of cortisol using cortisol monoclonal antibody (c-Mab) covalently immobilized on reduced graphene oxide (rGO) channel as electrical sensing element was demonstrated. Highly specific immune-recognition between the c-Mab and the cortisol was identified and characterized on a basis of resistance change at the rGO channel based chemiresistor sensor achieving the limit of detection of 10pg/mL (27.6 pM). In addition, cortisol concentrations of real human salivary sample and buffer solution of rat adrenal gland acute slices, which could secret the cortisol induced by adrenocorticotropic hormone (ACTH), were directly measured by the chemiresistor corresponding to the specific sensing of the cortisol...
July 11, 2017: Biosensors & Bioelectronics
https://www.readbyqxmd.com/read/28727446/reductive-outer-sphere-single-electron-transfer-is-an-exception-rather-than-the-rule-in-natural-and-engineered-chlorinated-ethene-dehalogenation
#19
Benjamin Heckel, Stefan Cretnik, Sarah Kliegman, Orfan Shouakar-Stash, Kristopher McNeill, Martin Elsner
Chlorinated ethenes (CEs) such as perchloroethylene, trichloroethylene and dichloroethylene are notorious groundwater contaminants. Although reductive dehalogenation is key to their environmental and engineered degradation, underlying reaction mechanisms remain elusive. Outer-sphere reductive single electron transfer (OS-SET) has been proposed for such different processes as Vitamin B12-dependent biodegradation and zero-valent metal-mediated dehalogenation. Compound-specific isotope effect (13C/12C, 37Cl/35Cl) analysis offers a new opportunity to test these hypotheses...
July 20, 2017: Environmental Science & Technology
https://www.readbyqxmd.com/read/28727416/in-situ-electrochemical-sensing-and-real-time-monitoring-live-cells-based-on-freestanding-nanohybrid-paper-electrode-assembled-from-3d-functionalized-graphene-framework
#20
Yan Zhang, Jian Xiao, Qi-Ying Lv, Lu Wang, Xulin Dong, Muhammad Asif, Jinghua Ren, Wenshan He, Yimin Sun, Fei Xiao, Shuai Wang
In this work, we develop a new type of freestanding nanohybrid paper electrode assembled from 3D ionic liquid (IL) functionalized graphene framework (GF) decorated by gold nanoflowers (AuNFs), and explore its practical application in in-situ electrochemical sensing of live breast cell samples by real-time tracking biomarker H2O2 released from cells. The AuNFs modified IL functionalized GF (AuNFs/IL-GF) was synthesized via a facile and efficient dopamine assisted one-pot self-assembly strategy. The as-obtained nanohybrid assembly exhibits a typical 3D hierarchical porous structure, where the highly active electrocatalyst AuNFs are well dispersed on IL-GF scaffold...
July 20, 2017: ACS Applied Materials & Interfaces
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