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Zero Quantum Coherence

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https://www.readbyqxmd.com/read/27892567/high-resolution-two-field-nuclear-magnetic-resonance-spectroscopy
#1
Samuel F Cousin, Cyril Charlier, Pavel Kadeřávek, Thorsten Marquardsen, Jean-Max Tyburn, Pierre-Alain Bovier, Simone Ulzega, Thomas Speck, Dirk Wilhelm, Frank Engelke, Werner Maas, Dimitrios Sakellariou, Geoffrey Bodenhausen, Philippe Pelupessy, Fabien Ferrage
Nuclear magnetic resonance (NMR) is a ubiquitous branch of spectroscopy that can explore matter at the scale of an atom. Significant improvements in sensitivity and resolution have been driven by a steady increase of static magnetic field strengths. However, some properties of nuclei may be more favourable at low magnetic fields. For example, transverse relaxation due to chemical shift anisotropy increases sharply at higher magnetic fields leading to line-broadening and inefficient coherence transfers. Here, we present a two-field NMR spectrometer that permits the application of rf-pulses and acquisition of NMR signals in two magnetic centres...
November 28, 2016: Physical Chemistry Chemical Physics: PCCP
https://www.readbyqxmd.com/read/27886234/expedited-holonomic-quantum-computation-via-net-zero-energy-cost-control-in-decoherence-free-subspace
#2
P V Pyshkin, Da-Wei Luo, Jun Jing, J Q You, Lian-Ao Wu
Holonomic quantum computation (HQC) may not show its full potential in quantum speedup due to the prerequisite of a long coherent runtime imposed by the adiabatic condition. Here we show that the conventional HQC can be dramatically accelerated by using external control fields, of which the effectiveness is exclusively determined by the integral of the control fields in the time domain. This control scheme can be realized with net zero energy cost and it is fault-tolerant against fluctuation and noise, significantly relaxing the experimental constraints...
November 25, 2016: Scientific Reports
https://www.readbyqxmd.com/read/27857400/controlling-collective-spontaneous-emission-with-plasmonic-waveguides
#3
Ying Li, Christos Argyropoulos
We demonstrate a plasmonic route to control the collective spontaneous emission of two-level quantum emitters. Superradiance and subradiance effects are observed over distances comparable to the operating wavelength inside plasmonic nanochannels. These plasmonic waveguides can provide an effective epsilon-near-zero operation in their cut-off frequency and Fabry-Pérot resonances at higher frequencies. The related plasmonic resonant modes are found to efficiently enhance the constructive (superradiance) or destructive (subradiance) interference between different quantum emitters located inside the waveguides...
November 14, 2016: Optics Express
https://www.readbyqxmd.com/read/27802628/effects-of-dynamic-disorder-on-exciton-migration-quantum-diffusion-coherences-and-energy-transfer
#4
Rajesh Dutta, Biman Bagchi
We study excitation transfer and migration in a one-dimensional lattice characterized by dynamic disorder. The diagonal and off-diagonal energy disorders arise from the coupling of system and bath. We consider both same bath (when baths are spatially correlated) and independent bath (when baths are completely uncorrelated) limits. In the latter case, all diagonal and off-diagonal bath coupling elements fluctuate independently of each other and the dynamics is complicated. We obtain time dependent population distribution by solving Kubo's quantum stochastic Liouville equation...
October 28, 2016: Journal of Chemical Physics
https://www.readbyqxmd.com/read/27727150/transport-shot-noise-and-topology-in-ac-driven-dimer-arrays
#5
Michael Niklas, Mónica Benito, Sigmund Kohler, Gloria Platero
We analyze an AC-driven dimer chain connected to a strongly biased electron source and drain. It turns out that the resulting transport exhibits fingerprints of topology. They are particularly visible in the driving-induced current suppression and the Fano factor. Thus, shot noise measurements provide a topological phase diagram as a function of the driving parameters. The observed phenomena can be explained physically by a mapping to an effective time-independent Hamiltonian and the emergence of edge states...
November 11, 2016: Nanotechnology
https://www.readbyqxmd.com/read/27574915/isolated-ground-state-vibrational-coherence-measured-by-fifth-order-single-shot-two-dimensional-electronic-spectroscopy
#6
William O Hutson, Austin P Spencer, Elad Harel
Vibrations play a critical role in many photochemical and photophysical processes in which excitations reside on the electronically excited state. However, difficulty in assigning signals from spectroscopic measurements uniquely to a specific electronic state, ground or otherwise, has exposed limitations to their physical interpretation. Here, we demonstrate the selective excitation of vibrational coherences on the ground electronic state through impulsive Raman scattering, whose weak fifth-order signal is resonantly enhanced by coupling to strong electronic transitions...
September 15, 2016: Journal of Physical Chemistry Letters
https://www.readbyqxmd.com/read/27193936/geometric-spin-echo-under-zero-field
#7
Yuhei Sekiguchi, Yusuke Komura, Shota Mishima, Touta Tanaka, Naeko Niikura, Hideo Kosaka
Spin echo is a fundamental tool for quantum registers and biomedical imaging. It is believed that a strong magnetic field is needed for the spin echo to provide long memory and high resolution, since a degenerate spin cannot be controlled or addressed under a zero magnetic field. While a degenerate spin is never subject to dynamic control, it is still subject to geometric control. Here we show the spin echo of a degenerate spin subsystem, which is geometrically controlled via a mediating state split by the crystal field, in a nitrogen vacancy centre in diamond...
2016: Nature Communications
https://www.readbyqxmd.com/read/27181882/evidence-of-weak-localization-in-quantum-interference-effects-observed-in-epitaxial-la0-7sr0-3mno3-ultrathin-films
#8
Wei Niu, Ming Gao, Xuefeng Wang, Fengqi Song, Jun Du, Xinran Wang, Yongbing Xu, Rong Zhang
Quantum interference effects (QIEs) dominate the appearance of low-temperature resistivity minimum in colossal magnetoresistance manganites. The T(1/2) dependent resistivity under high magnetic field has been evidenced as electron-electron (e-e) interaction. However, the evidence of the other source of QIEs, weak localization (WL), still remains insufficient in manganites. Here we report on the direct experimental evidence of WL in QIEs observed in the single-crystal La0.7Sr0.3MnO3 (LSMO) ultrathin films deposited by laser molecular beam epitaxy...
2016: Scientific Reports
https://www.readbyqxmd.com/read/27127238/large-optical-nonlinearity-of-indium-tin-oxide-in-its-epsilon-near-zero-region
#9
M Zahirul Alam, Israel De Leon, Robert W Boyd
Nonlinear optical phenomena are crucial for a broad range of applications, such as microscopy, all-optical data processing, and quantum information. However, materials usually exhibit a weak optical nonlinearity even under intense coherent illumination. We report that indium tin oxide can acquire an ultrafast and large intensity-dependent refractive index in the region of the spectrum where the real part of its permittivity vanishes. We observe a change in the real part of the refractive index of 0.72 ± 0...
May 13, 2016: Science
https://www.readbyqxmd.com/read/26979686/high-resolution-nuclear-magnetic-resonance-measurements-in-inhomogeneous-magnetic-fields-a-fast-two-dimensional-j-resolved-experiment
#10
Yuqing Huang, Yung-Ya Lin, Shuhui Cai, Yu Yang, Huijun Sun, Yanqin Lin, Zhong Chen
High spectral resolution in nuclear magnetic resonance (NMR) is a prerequisite for achieving accurate information relevant to molecular structures and composition assignments. The continuous development of superconducting magnets guarantees strong and homogeneous static magnetic fields for satisfactory spectral resolution. However, there exist circumstances, such as measurements on biological tissues and heterogeneous chemical samples, where the field homogeneity is degraded and spectral line broadening seems inevitable...
March 14, 2016: Journal of Chemical Physics
https://www.readbyqxmd.com/read/26772564/site-resolved-multiple-quantum-filtered-correlations-and-distance-measurements-by-magic-angle-spinning-nmr-theory-and-applications-to-spins-with-weak-to-vanishing-quadrupolar-couplings
#11
U Eliav, A Haimovich, A Goldbourt
We discuss and analyze four magic-angle spinning solid-state NMR methods that can be used to measure internuclear distances and to obtain correlation spectra between a spin I = 1/2 and a half-integer spin S > 1/2 having a small quadrupolar coupling constant. Three of the methods are based on the heteronuclear multiple-quantum and single-quantum correlation experiments, that is, high rank tensors that involve the half spin and the quadrupolar spin are generated. Here, both zero and single-quantum coherence of the half spins are allowed and various coherence orders of the quadrupolar spin are generated, and filtered, via active recoupling of the dipolar interaction...
January 14, 2016: Journal of Chemical Physics
https://www.readbyqxmd.com/read/26739626/employing-forbidden-transitions-as-qubits-in-a-nuclear-spin-free-chromium-complex
#12
Majed S Fataftah, Joseph M Zadrozny, Scott C Coste, Michael J Graham, Dylan M Rogers, Danna E Freedman
The implementation of quantum computation (QC) would revolutionize scientific fields ranging from encryption to quantum simulation. One intuitive candidate for the smallest unit of a quantum computer, a qubit, is electronic spin. A prominent proposal for QC relies on high-spin magnetic molecules, where multiple transitions between the many MS levels are employed as qubits. Yet, over a decade after the original notion, the exploitation of multiple transitions within a single manifold for QC remains unrealized in these high-spin species due to the challenge of accessing forbidden transitions...
February 3, 2016: Journal of the American Chemical Society
https://www.readbyqxmd.com/read/26723664/establishing-resolution-improved-nmr-spectroscopy-in-high-magnetic-fields-with-unknown-spatiotemporal-variations
#13
Zhiyong Zhang, Pieter E S Smith, Shuhui Cai, Zhenyao Zheng, Yulan Lin, Zhong Chen
A half-century quest for higher magnetic fields has been an integral part of the progress undergone in the Nuclear Magnetic Resonance (NMR) study of materials' structure and dynamics. Because 2D NMR relies on systematic changes in coherences' phases as a function of an encoding time varied over a series of independent experiments, it generally cannot be applied in temporally unstable fields. This precludes most NMR methods from being used to characterize samples situated in hybrid or resistive magnets that are capable of achieving extremely high magnetic field strength...
December 28, 2015: Journal of Chemical Physics
https://www.readbyqxmd.com/read/26682627/how-quantum-entanglement-in-dna-synchronizes-double-strand-breakage-by-type-ii-restriction-endonucleases
#14
P Kurian, G Dunston, J Lindesay
Macroscopic quantum effects in living systems have been studied widely in pursuit of fundamental explanations for biological energy transport and sensing. While it is known that type II endonucleases, the largest class of restriction enzymes, induce DNA double-strand breaks by attacking phosphodiester bonds, the mechanism by which simultaneous cutting is coordinated between the catalytic centers remains unclear. We propose a quantum mechanical model for collective electronic behavior in the DNA helix, where dipole-dipole oscillations are quantized through boundary conditions imposed by the enzyme...
February 21, 2016: Journal of Theoretical Biology
https://www.readbyqxmd.com/read/26595331/revealing-giant-internal-magnetic-fields-due-to-spin-fluctuations-in-magnetically-doped-colloidal-nanocrystals
#15
William D Rice, Wenyong Liu, Thomas A Baker, Nikolai A Sinitsyn, Victor I Klimov, Scott A Crooker
Strong quantum confinement in semiconductors can compress the wavefunctions of band electrons and holes to nanometre-scale volumes, significantly enhancing interactions between themselves and individual dopants. In magnetically doped semiconductors, where paramagnetic dopants (such as Mn(2+), Co(2+) and so on) couple to band carriers via strong sp-d spin exchange, giant magneto-optical effects can therefore be realized in confined geometries using few or even single impurity spins. Importantly, however, thermodynamic spin fluctuations become increasingly relevant in this few-spin limit...
February 2016: Nature Nanotechnology
https://www.readbyqxmd.com/read/26551122/dynamical-quasicondensation-of-hard-core-bosons-at-finite-momenta
#16
L Vidmar, J P Ronzheimer, M Schreiber, S Braun, S S Hodgman, S Langer, F Heidrich-Meisner, I Bloch, U Schneider
Long-range order in quantum many-body systems is usually associated with equilibrium situations. Here, we experimentally investigate the quasicondensation of strongly interacting bosons at finite momenta in a far-from-equilibrium case. We prepare an inhomogeneous initial state consisting of one-dimensional Mott insulators in the center of otherwise empty one-dimensional chains in an optical lattice with a lattice constant d. After suddenly quenching the trapping potential to zero, we observe the onset of coherence in spontaneously forming quasicondensates in the lattice...
October 23, 2015: Physical Review Letters
https://www.readbyqxmd.com/read/26520505/analyzing-the-special-pfg-signal-attenuation-behavior-of-intermolecular-mqc-via-the-effective-phase-shift-diffusion-equation-method
#17
Guoxing Lin
Inter-molecular multiple quantum coherence (iMQC) has important applications in NMR and MRI. However, the current theoretical methods still have some difficulties in analyzing the behavior of iMQC signal attenuation of pulsed field gradient diffusion experiments. In this paper, the iMQC diffusion experiments were analyzed by an effective phase shift diffusion equation (EPSDE) method, which is based on the idea that the accumulating phase shift (APS) can be viewed as the result of a diffusion process in virtual phase space (VPS) with effective diffusion coefficient K(2)(t) D (rad(2)/s) where K(t)=∫0 (t)γg(t')dt' is a wavenumber and D is the physical diffusion coefficient of the spin carrier in the real space...
October 28, 2015: Journal of Chemical Physics
https://www.readbyqxmd.com/read/26483465/pressure-tuned-quantum-criticality-in-the-antiferromagnetic-kondo-semimetal-ceni2-%C3%AE-as2
#18
Yongkang Luo, F Ronning, N Wakeham, Xin Lu, Tuson Park, Z-A Xu, J D Thompson
The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers...
November 3, 2015: Proceedings of the National Academy of Sciences of the United States of America
https://www.readbyqxmd.com/read/26434582/enhancement-of-the-si-p-n-diode-nir-photoresponse-by-embedding-%C3%AE-fesi2-nanocrystallites
#19
A V Shevlyagin, D L Goroshko, E A Chusovitin, K N Galkin, N G Galkin, A K Gutakovskii
By using solid phase epitaxy of thin Fe films and molecular beam epitaxy of Si, a p(+)-Si/p-Si/β-FeSi2 nanocrystallites/n-Si(111) diode structure was fabricated. Transmission electron microscopy data confirmed a well-defined multilayered structure with embedded nanocrystallites of two typical sizes: 3-4 and 15-20 nm, and almost coherent epitaxy of the nanocrystallites with the Si matrix. The diode at zero bias conditions exhibited a current responsivity of 1.7 mA/W, an external quantum efficiency of about 0...
2015: Scientific Reports
https://www.readbyqxmd.com/read/26417918/picosecond-dynamics-of-excitonic-magnetic-polarons-in-colloidal-diffusion-doped-cd-1-x-mn-x-se-quantum-dots
#20
Heidi D Nelson, Liam R Bradshaw, Charles J Barrows, Vladimir A Vlaskin, Daniel R Gamelin
Spontaneous magnetization is observed at zero magnetic field in photoexcited colloidal Cd(1-x)Mn(x)Se (x = 0.13) quantum dots (QDs) prepared by diffusion doping, reflecting strong Mn(2+)-exciton exchange coupling. The picosecond dynamics of this phenomenon, known as an excitonic magnetic polaron (EMP), are examined using a combination of time-resolved photoluminescence, magneto-photoluminescence, and Faraday rotation (TRFR) spectroscopies, in conjunction with continuous-wave absorption, magnetic circular dichroism (MCD), and magnetic circularly polarized photoluminescence (MCPL) spectroscopies...
November 24, 2015: ACS Nano
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