keyword
https://read.qxmd.com/read/38563938/first-measurement-of-discrimination-between-helium-and-electron-recoils-in-liquid-xenon-for-low-mass-dark-matter-searches
#21
JOURNAL ARTICLE
S J Haselschwardt, R Gibbons, H Chen, S Kravitz, A Manalaysay, Q Xia, W H Lippincott, P Sorensen
We report the first measurement of discrimination between low-energy helium recoils and electron recoils in liquid xenon. This result is relevant to proposed low-mass dark matter searches which seek to dissolve light target nuclei in the active volume of liquid-xenon time projection chambers. Low-energy helium recoils were produced by degrading α particles from ^{210}Po with a gold foil situated on the cathode of a liquid xenon time-projection chamber. The resulting population of helium recoil events is well separated from electron recoils and is also offset from the expected position of xenon nuclear recoil events...
March 15, 2024: Physical Review Letters
https://read.qxmd.com/read/38563716/a-hermetic-on-cryostat-helium-source-for-low-temperature-experiments
#22
JOURNAL ARTICLE
K E Castoria, H Byeon, J Theis, N R Beysengulov, E O Glen, G Koolstra, M Sammon, S A Lyon, J Pollanen, D G Rees
We describe a helium source cell for use in cryogenic experiments that is hermetically sealed in situ on the cold plate of a cryostat. The source cell is filled with helium gas at room temperature and, subsequently, sealed using a cold weld crimping tool before the cryostat is closed and cooled down. At low temperatures, the helium condenses and collects in a connected experimental volume, as monitored via the frequency response of a planar superconducting resonator device sensitive to small amounts of liquid helium...
April 1, 2024: Review of Scientific Instruments
https://read.qxmd.com/read/38557888/electric-charging-effects-on-insulating-surfaces-in-cryogenic-liquids
#23
JOURNAL ARTICLE
Wolfgang Korsch, Mark Broering, Ashok Timsina, Kent K H Leung, Joshua Abney, Dmitry Budker, Bradley W Filippone, Jiachen He, Suman Kandu, Mark McCrea, Murchhana Roy, Christopher Swank, Weijun Yao
This paper presents a new technique to study the adsorption and desorption of ions and electrons on insulating surfaces in the presence of strong electric fields in cryoliquids. The experimental design consists of a compact cryostat coupled with a sensitive electro-optical Kerr device to monitor the stability of the electric fields. The behavior of nitrogen and helium ions on a poly(methyl methacrylate) (PMMA) surface was compared to a PMMA surface coated with a mixture of deuterated polystyrene and deuterated polybutadiene...
April 1, 2024: Review of Scientific Instruments
https://read.qxmd.com/read/38557840/structure-determination-of-alkali-trimers-on-helium-nanodroplets-through-laser-induced-coulomb-explosion
#24
JOURNAL ARTICLE
Lorenz Kranabetter, Henrik H Kristensen, Constant A Schouder, Henrik Stapelfeldt
Alkali trimers, Ak3, located on the surface of He nanodroplets are triply ionized following multiphoton absorption from an intense femtosecond laser pulse, leading to fragmentation into three correlated Ak+ ions. Combining the information from threefold covariance analysis of the emission direction of the fragment ions and their kinetic energy distributions P(Ekin), we find that Na3, K3, and Rb3 have an equilateral triangular structure, corresponding to that of the lowest lying quartet state A2'4, and determine the equilibrium bond distance Req(Na3) = 4...
April 7, 2024: Journal of Chemical Physics
https://read.qxmd.com/read/38551487/chemical-aristocracy-he-3-dication-and-analogous-noble-gas-exclusive-covalent-compounds
#25
JOURNAL ARTICLE
Lucas Araujo, Felipe Fantuzzi, Thiago M Cardozo
Herein, we predict the first set of covalently bonded triatomic molecular compounds composed exclusively of noble gases. Using a combination of double-hybrid DFT, CCSD(T), and MRCI+Q calculations and a range of bonding analyses, we explored a set of 270 doubly charged triatomics, which included various combinations of noble gases and main group elements. This extensive exploration uncovered nine noble-gas-exclusive covalent compounds incorporating helium, neon, argon, or combinations thereof, exemplified by cases such as He3 2+ and related systems...
March 29, 2024: Journal of Physical Chemistry Letters
https://read.qxmd.com/read/38545616/adsorption-of-n-he-and-ne-on-cge-nanoribbons-for-sensing-and-optoelectronic-applications
#26
JOURNAL ARTICLE
Hoang Van Ngoc
Research into nanomaterials yields numerous exceptional applications in contemporary science and technology. The subject of this investigation is a one-dimensional nanostructure, six atoms wide, featuring hydrogen-functionalized edges. The theoretical foundation of this study relies on Density Functional Theory (DFT) and is executed through the utilization of the Vienna Ab initio Simulation Package (VASP). The outcomes demonstrate the stability of adsorption configurations, along with the preservation of a hexagonal honeycomb lattice...
March 2024: Royal Society Open Science
https://read.qxmd.com/read/38540286/cold-atmospheric-plasma-improves-the-colonization-of-titanium-with-primary-human-osteoblasts-an-in-vitro-study
#27
JOURNAL ARTICLE
Madline P Gund, Jusef Naim, Antje Lehmann, Matthias Hannig, Markus Lange, Axel Schindler, Stefan Rupf
Several studies have shown that cold atmospheric plasma (CAP) treatment can favourably modify titanium surfaces to promote osteoblast colonization. The aim of this study was to investigate the initial attachment of primary human osteoblasts to plasma-treated titanium. Micro-structured titanium discs were treated with cold atmospheric plasma followed by the application of primary human osteoblasts. The microwave plasma source used in this study uses helium as a carrier gas and was developed at the Leibniz Institute for Surface Modification in Leipzig, Germany...
March 18, 2024: Biomedicines
https://read.qxmd.com/read/38538354/-effects-of-helium-oxygen-mechanical-ventilation-on-inflammatory-response-of-diseased-lung-segments-and-diaphragm-function-in-patients-with-pneumonia
#28
JOURNAL ARTICLE
Decai Ren, Lili Zhou, Chengqing Zheng, Shanmin Xie, Ranjie Yu
OBJECTIVE: To investigate the clinical effect of helium-oxygen mechanical ventilation on inflammation of the diseased lung segment and diaphragm function in patients with acute respiratory distress syndrome (ARDS) caused by pneumonia who suffered difficulty weaning from mechanical ventilation. METHODS: A prospective controlled study was conducted. A total of 40 patients with ARDS caused by pneumonia and requiring tracheal intubation with difficulty weaning from mechanical ventilation, admitted to the department of critical care medicine in Pingtan Branch of Fujian Medical University Union Hospital from October 2020 to December 2021 were enrolled...
March 2024: Zhonghua Wei Zhong Bing Ji Jiu Yi Xue
https://read.qxmd.com/read/38533827/doubly-charged-dimers-and-trimers-of-heavy-noble-gases
#29
JOURNAL ARTICLE
Gabriel Schöpfer, Stefan Bergmeister, Milan Ončák, Ianessa Stromberg, Masoomeh Mahmoodi-Darian, Paul Scheier, Olof Echt, Elisabeth Gruber
Many doubly charged heteronuclear dimers are metastable or even thermodynamically stable with respect to charge separation. Homonuclear dicationic dimers, however, are more difficult to form. He2 2+ was the first noble gas dimer predicted to be metastable and, decades later, observed. Ne2 2+ is the only other dicationic noble gas dimer that has been detected so far. Here, we present a novel approach to form fragile dicationic species, by post-ionization of singly charged ions that are embedded in helium nanodroplets (HNDs)...
March 27, 2024: Physical Chemistry Chemical Physics: PCCP
https://read.qxmd.com/read/38529414/sustainable-power-generation-through-solar-driven-integration-of-brayton-and-transcritical-co-2-cycles-a-comprehensive-3e-energy-exergy-and-exergoenvironmental-evaluation
#30
JOURNAL ARTICLE
Yunis Khan, Roshan Raman, Zafar Said, Hakan Caliskan, Hiki Hong
Solar power tower technology has strong potential among the other concentration solar power techniques for large power generation. Therefore, it is necessary to make a new and efficient power conversion system for utilizing the solar power tower system. In present research, a novel combined cycle is proposed to generate power for the application of the solar power tower. The pre-compression configuration of the Brayton cycle is used as a topping cycle in which helium is taken as the working fluid. The transcritical CO2 cycle is used as bottoming cycle for using the waste heat...
February 2024: Global Challenges
https://read.qxmd.com/read/38518314/femtosecond-collisional-dissipation-of-vibrating-d_-2-in-helium-nanodroplets
#31
JOURNAL ARTICLE
Junjie Qiang, Lianrong Zhou, Yigeng Peng, Chao Yu, Peifen Lu, Shengzhe Pan, Chenxu Lu, Gang Chen, Ruifeng Lu, Wenbin Zhang, Jian Wu
We explored the collision-induced vibrational decoherence of singly ionized D_{2} molecules inside a helium nanodroplet. By using the pump-probe reaction microscopy with few-cycle laser pulses, we captured in real time the collision-induced ultrafast dissipation of vibrational nuclear wave packet dynamics of D_{2}^{+} ion embedded in the droplet. Because of the strong coupling of excited molecular cations with the surrounding solvent, the vibrational coherence of D_{2}^{+} in the droplet interior only lasts for a few vibrational periods and completely collapses within 140 fs...
March 8, 2024: Physical Review Letters
https://read.qxmd.com/read/38517257/method-of-kinetic-energy-reconstruction-from-time-of-flight-mass-spectra
#32
JOURNAL ARTICLE
A Ngai, K Dulitz, S Hartweg, J C Franz, M Mudrich, F Stienkemeier
We present a method for the reconstruction of ion kinetic energy distributions from ion time-of-flight mass spectra through ion trajectory simulations. In particular, this method is applicable to complicated spectrometer geometries with largely anisotropic ion collection efficiencies. A calibration procedure using a single ion mass peak allows the accurate determination of parameters related to the spectrometer calibration, experimental alignment, and instrument response function, which improves the agreement between simulations and experiment...
March 1, 2024: Review of Scientific Instruments
https://read.qxmd.com/read/38516916/coincidence-measurements-of-photodouble-ionization-of-benzene-and-thiophene
#33
JOURNAL ARTICLE
Nicholas L Wong, Jason Howard, Ben Delaney, Emma Sokell, Paola Bolognesi, Lorenzo Avaldi
Photodouble ionization (PDI) triple-differential cross sections (TDCSs) of benzene and thiophene have been measured in electron-electron coincidence experiments under 10-10 eV and 20-20 eV equal energy sharing conditions. A multi-Gaussian fit method has been employed to characterize the TDCSs. The trends and features observed for benzene and thiophene do highlight differences with helium most likely from molecular PDI contributions to the TDCS. A comparison with the well-known helium PDI TDCS for equal energy sharing conditions [Avaldi and Huetz J...
March 22, 2024: Physical Chemistry Chemical Physics: PCCP
https://read.qxmd.com/read/38511250/infrared-laser-stark-spectroscopy-of-methyl-fluoride-in-4he-nanodroplets
#34
JOURNAL ARTICLE
Paul Raston, Gary E Douberly
We measured the rotationally resolved infrared spectra of helium solvated methyl fluoride at 3 μm and 10 μm, wherein lies C-H and C-F stretching bands, respectively. The linewidths (FWHM) were found to increase with increasing vibrational energy and range from 0.002 cm-1 in the v3 band (C-F stretch) at ~1047 cm-1, to 0.65 cm-1 in the v4 band (asymmetric C-H stretch) at ~2997 cm-1. In between these two bands we observed the lower and upper components of the Fermi triad bands (ν1/2ν2/2ν5) at ~2859 and ~2961 cm-1...
March 21, 2024: Chemphyschem: a European Journal of Chemical Physics and Physical Chemistry
https://read.qxmd.com/read/38509446/in-situ-helium-isotope-microimaging-of-meteorites
#35
JOURNAL ARTICLE
Ken-Ichi Bajo, Noriyuki Kawasaki, Isao Sakaguchi, Taku T Suzuki, Satoru Itose, Miyuki Matsuya, Morio Ishihara, Kiichiro Uchino, Hisayoshi Yurimoto
Isotope imaging is commonly used to investigate the localization of trace elements and their isotopes. In situ noble gas analysis of meteorites revealed the distribution of primordial noble gases that were trapped in the building blocks of asteroids and planets during the early stage of the solar system evolution. Solar wind noble gases are among the primordial gases present in meteorites and were trapped through exposure to solar wind. Micrometer-resolution in situ noble gas analysis has not been achieved due to the lack of sensitivity and spatial resolution...
March 20, 2024: Analytical Chemistry
https://read.qxmd.com/read/38509373/rotating-curved-spacetime-signatures-from-a-giant-quantum-vortex
#36
JOURNAL ARTICLE
Patrik Švančara, Pietro Smaniotto, Leonardo Solidoro, James F MacDonald, Sam Patrick, Ruth Gregory, Carlo F Barenghi, Silke Weinfurtner
Gravity simulators1 are laboratory systems in which small excitations such as sound2 or surface waves3,4 behave as fields propagating on a curved spacetime geometry. The analogy between gravity and fluids requires vanishing viscosity2-4 , a feature naturally realized in superfluids such as liquid helium or cold atomic clouds5-8 . Such systems have been successful in verifying key predictions of quantum field theory in curved spacetime7-11 . In particular, quantum simulations of rotating curved spacetimes indicative of astrophysical black holes require the realization of an extensive vortex flow12 in superfluid systems...
March 20, 2024: Nature
https://read.qxmd.com/read/38507913/the-first-deep-rebreather-dive-using-hydrogen-case-report
#37
Richard J Harris, Craig J Challen, Simon J Mitchell
Bounce diving with rapid descents to very deep depths may provoke the high-pressure neurological syndrome (HPNS). The strategy of including small fractions of nitrogen in the respired gas to produce an anti-HPNS narcotic effect increases the gas density which may exceed recommended guidelines. In 2020 the 'Wetmules' dive team explored the Pearse Resurgence cave (New Zealand) to 245 m breathing trimix (approximately 4% oxygen, 91% helium and 5% nitrogen). Despite the presence of nitrogen, one diver experienced HPNS tremors beyond 200 m...
March 31, 2024: Diving and Hyperbaric Medicine: the Journal of the South Pacific Underwater Medicine Society
https://read.qxmd.com/read/38506993/a-static-headspace-gas-chromatography-method-for-quantitation-of-residual-solvents-in-nanoformulations
#38
JOURNAL ARTICLE
Krishna Kattel, Jeffrey D Clogston
Various organic solvents are widely used in the manufacturing, processing, and purification of drug substances, drug products, formulations, excipients, etc. These solvents must be removed to the lowest amount permitted, as they do not possess any therapeutic advantages and may cause undesirable toxicities. Therefore, a rapid and sensitive analytical method for the quantitation of residual solvents is needed. The following chapter presents a static headspace gas chromatographic (HSGC) method for determining the concentration of common residual solvents in various nanoformulations...
2024: Methods in Molecular Biology
https://read.qxmd.com/read/38502316/exploring-the-potential-of-metal-organic-frameworks-for-cryogenic-helium-based-gas-gap-heat-switches-via-high-throughput-computational-screening
#39
JOURNAL ARTICLE
Lingxiao Qin, Haishan Cao
With the advantages of a long lifetime and high reliability, gas gap heat switches (GGHSs) are attractive in many thermal management applications, especially in space-borne cryogenic systems. The performance of a GGHS is significantly affected by the adsorption characteristics of the adsorbent in the sorption pump. Compared with the commonly used adsorbent in the GGHSs (activated carbon), metal-organic frameworks (MOFs) have larger surface areas, higher pore volumes, and exceptional tunability, which motivates this study to explore their potential for application in cryogenic GGHSs...
March 19, 2024: ACS Applied Materials & Interfaces
https://read.qxmd.com/read/38501477/the-associative-ionization-of-n-2p-o-3p
#40
JOURNAL ARTICLE
Nicholas S Shuman, Thomas M Miller, Shaun G Ard, Albert A Viggiano
The rate constant of the associative ionization reaction N(2P) + O(3P) → NO+ + e- was measured using a flow tube apparatus. A flowing afterglow source was used to produce an ion/electron plasma containing a mixture of ions, including N2+, N3+, and N4+. Dissociative recombination of these species produced a population of nitrogen atoms, including N(2P). Charged species were rejected from the flow tube using an electrostatic grid, subsequent to which oxygen atoms were introduced, produced either using a discharge of helium and oxygen or via the titration of nitrogen atoms with NO...
March 21, 2024: Journal of Chemical Physics
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